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Frequency Quadrupling

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Definition: the phenomenon that an input laser beam generates a beam with four times the optical frequency

Frequency quadrupling is a process of nonlinear frequency conversion where the resulting optical frequency is four times that of the input laser beam, which means that the wavelength is reduced by a factor of 4. This can be accomplished with two sequential frequency doublers (Figure 1).

frequency quadrupling

Figure 1: A typical configuration for frequency quadrupling: an infrared input beam at 1064 nm generates a green 532-nm wave in a first frequency doubler, and a second frequency doubler converts this to light at 266 nm.

A commonly used frequency quadrupling configuration begins with a continuous-wave or pulsed Nd:YAG laser at 1064 nm for generating 532-nm light in a first frequency doubler stage (based e.g. on LBO) and then 266 nm in a second stage (based e.g. on CLBO). Such ultraviolet light is useful e.g. to pump a dye laser or an optical parametric oscillator, for Raman spectroscopy in flames, or for material processing, e.g. the writing of fiber Bragg gratings.

Bibliography

 [1]J. Reintjes and R. C. Eckardt, "Efficient harmonic generation from 532 to 266 nm in ADP and KD*P", Appl. Phys. Lett. 30, 91 (1977)
[2]D. Bruneau et al., "Fourth harmonic generation of a large-aperture Nd:glass laser", Appl. Opt. 24 (22), 3740 (1985)
[3]B. A. Hooper et al., "Fourth-harmonic generation in a single lithium niobate-crystal with cascaded second-harmonic generation", Appl. Opt. 33 (30), 6980 (1994)
[4]M. Oka et al., "All solid state continuous-wave frequency-quadrupled Nd:YAG laser", IEEE J. Sel. Top. Quantum Electron. 1, 859 (1995)
[5]J. Knittel and A. H. Kung, "Fourth harmonic generation in a resonant ring cavity", IEEE J. Quantum Electron. 33 (11), 2021 (1997)
[6]T. Kojima et al., "20-W ultraviolet-beam generation by fourth-harmonic generation of an all-solid-state laser", Opt. Lett. 25 (1), 58 (2000)
 [7]T. Südmeyer et al., "Efficient 2nd and 4th harmonic generation of a single-frequency, continuous-wave fiber amplifier", Opt. Express 16 (3), 1546 (2008)

See also: frequency doubling, frequency tripling, nonlinear frequency conversion, ultraviolet lasers

Category: nonlinear optics

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