Laser-induced Breakdown | previous | next | feedback |
Definition: a kind of spark, initiated by intense laser light
From electrical engineering, it is known that for high electric field strengths in air (under normal conditions roughly above 1 kV/mm) a breakdown can occur. This means that there is a kind of spark, and the air becomes electrically conducting. The mechanism behind this effect is based on the acceleration of free electrons to high energies so that collisions with air molecules can lead to secondary free carriers. This starts an avalanche process, during which appreciable densities of free carriers can be built up within a short time. A plasma is formed, which can have a significant electrical conductivity. The plasma can be maintained by further current flow, which generates additional free carriers.
Breakdown in air (and in other transparent media) can also be initiated by intense light, i.e., by electromagnetic waves with frequencies of hundreds of terahertz. The required high optical intensities can be reached in pulses as generated e.g. in a Q-switched laser (with nanosecond durations) or in a mode-locked laser and amplified in a regenerative amplifier (for pulse durations of picoseconds or femtoseconds). The required intensity for optical breakdown depends on the pulse duration. For example, for 1-ps pulses an optical intensity of ∼2⋅1013 W/cm2 is required.
Physical Mechanisms
The detailed mechanisms behind breakdown with optical pulses are quite different from those for static electric fields, also depend on the pulse duration. Particularly for femtosecond pulses, multiphoton ionization can efficiently generate free carriers in the initial phase of the pulse, followed by strong absorption by the generated plasma, which leads to further heating and ionization [2]. For long pulses, multiphoton ionization is less important, and the breakdown starts primarily from few carriers which are already present before the pulse. The random occurrence of such carriers makes optical breakdown less deterministic in the regime of longer pulses, whereas the damage threshold can be very well defined for femtosecond pulses.
Breakdown in Laser Machining
Optical breakdown can constitute a severe problem for laser machining (e.g. drilling holes with laser light), because it does not only extract energy from the beam before it reaches the target, but also tends to defocus the beam, with the effect that the mechanical quality of the achieved holes or cuts can be severely degraded. This happens particularly for pulse durations well below 1 ps, where breakdown easily occurs above the target – even when the focus is on the target, so that the optical intensities are lower above it. Colorful ring-like structures can occur due to nonlinear frequency conversion in the plasma; this phenomenon is called conical emission.
Although optical breakdown is often undesirable in laser machining, it can be used e.g. for machining transparent media such as glasses or polymers. There, the breakdown can modify the material structure through various effects and in this way modify the refractive index or the degree of transparency. Rather small structures (sometimes with dimensions below a micrometer) can be generated within a transparent medium when using ultrashort pulses (often with durations below 1 ps) and a strongly focused laser beam, where only in the focus the intensity is sufficient for modifying the material, while other parts of the work piece stay unaffected. When the focus is moved within a transparent medium, a waveguide can be created. This technique might be used e.g. for photonic integrated circuits. The use of very short pulses is essential, because only then the process is deterministic (see above).
Application in Spectroscopy
There is also a technique called laser-induced breakdown spectroscopy (LIBS) [4], where a laser pulse is used for generating a hot plasma at the surface of some test object, and spectroscopic investigation of the light emitted from the plasma is used for determining what chemical elements exist in the sample. Such techniques are currently developed e.g. for a mars exploration, where laser-induced breakdown spectroscopy should allow to rapidly analyze the composition of marsian rocks from a robotic vehicle over a distance of a several meters.
Bibliography
| [1] | C. DeMichelis, "Laser induced gas breakdown: a bibliographical review", IEEE J. Quantum Electron. 5 (4), 188 (1969) |
| [2] | D. Du et al., "Laser-induced breakdown by impact ionization in SiO2 with pulse widths from 7 ns to 150 fs", Appl. Phys. Lett. 64, 3071 (1994) |
| [3] | B. C. Stuart et al., "Laser-induced damage in dielectrics with nanosecond to sub-picosecond pulses", Phys. Rev. Lett. 74 (12), 2248 (1995) |
| [4] | D. A. Cremers and L. J. Radziemski, "Handbook of laser-induced breakdown spectroscopy", John Wiley & Sons, 2006, ISBN: 0470092998 |
See also: nonlinearities, waveguides, pulses
Category: physical foundations
