Saturable Absorbers

Definition: light absorbers with a degree of absorption which is decreases at high optical intensities

A saturable absorber is an optical component with a certain optical loss, which is reduced at high optical intensities. This can occur, e.g., in a medium with absorbing dopant ions, when a strong optical intensity leads to depletion of the ground state of these ions. Similar effects can occur in semiconductors, where excitation of electrons from the valence band into the conduction band reduces the absorption for photon energies just above the bandgap energy.

The main applications of saturable absorbers are passive mode locking and Q switching of lasers, i.e., the generation of short pulses. However, saturable absorbers are also useful for purposes of nonlinear filtering outside laser resonators, e.g. for cleaning up pulse shapes, and in optical signal processing.

Types of Saturable Absorbers

As different applications require saturable absorbers with very different parameters, different devices are used:

• Particularly for passive mode locking (but also for Q switching), semiconductor saturable absorber mirrors (also called SESAMs) are frequently used [5]. These are also suitable for passive Q switching, particularly at lower pulse energies.
• Other semiconductor saturable absorbers for mode locking or Q switching are based on quantum dots e.g. of lead sulfide (PbS) suspended in glasses [9].
• Thin layers of carbon nanotubes have been used for mode locking of lasers [11, 14, 15]. Such absorbers can exhit very broadband absorption features as are desirable for broadband lasers.
• In some mode-locked diode lasers, a saturable absorber section is created simply by not pumping that region. A faster recovery can be obtained by implanting nitrogen (N⁺) ions.
• Gallium arsenide (GaAs) is also sometimes used for passive Q switching of 1-μm lasers, even though the photon energy of these lasers is below the bandgap in that case. Certain crystal defects play an important role for the absorption.
• For passive Q switching of solid-state lasers in the 1-μm spectral region, Cr⁴⁺:YAG saturable absorber crystals are most popular [12]. (Cr:YAG crystals are also used as gain media → chromium-doped gain media.) For 1.3-μm lasers, V³⁺:YAG can be used [10], whereas Co²⁺:MgAl₂O₄ and some other cobalt-doped crystal materials can be used in the 1.5-μm spectral region. There are also laser crystals with an integrated saturable absorber dopant – for example, with Cr⁴⁺ in a Nd³⁺-doped laser crystal, such as Nd:Cr:YVO₄.
• In rare cases, saturable absorber materials are used in the form of optical fibers. For example, chromium, samarium or bismuth dopants can serve this function in Q-switched fiber lasers [13].

Artificial Saturable Absorbers

There are also various kinds of artificial saturable absorbers. These are devices which exhibit decreasing optical losses for higher intensities, but not actually exploiting saturable absorption. Such devices can be based on e.g.

• Kerr lensing combined with some kind of aperture (→ Kerr lens mode locking) [4]
• a nonlinear mirror device containing a frequency-doubling crystal, as sometimes used for passive mode locking of solid-state bulk lasers [2]
• a nonlinear fiber within an auxiliary resonator (→ additive-pulse mode locking) [7]
• nonlinear polarization rotation in a fiber, combined with a polarizing element, often used for passive mode locking of fiber lasers [8]
• a nonlinear fiber loop mirror, also used for mode locking of fiber lasers [3]
• an array of waveguides, exhibiting nonlinear coupling [16]

Properties of Saturable Absorbers

The most important properties of saturable absorbers are:

• The modulation depth is the maximum possible change in optical loss, specified in percent, for example.
• The non-saturable losses are the (typically unwanted) part of the losses which can not be saturated. This can result from defect centers in SESAMs, or from excited-state absorption in case of doped-insulator absorbers such as Cr⁴⁺:YAG.
• The recovery time is the decay time of the excitation after an exciting pulse. This should be very short for passive mode locking, but not too short for passive Q switching.
• The saturation fluence is the fluence (energy per unit area) it takes to reduce the initial value to 1/e (≈ 37%) of its initial value. A large saturation fluence can often be compensated by using a tightly focused beam in the absorber.
• The saturation energy is the saturation fluence times the mode area. Strong saturation occurs for incident optical energies above the saturation energy.
• The saturation intensity is the optical intensity (power per unit area) that it takes in a steady state to reduce the absorption to half of its unbleached value. Note that many absorbers are never operated in the steady state, and might even be destroyed when trying to keep them saturated over longer times.
• The saturation power is the saturation intensity times the mode area.
• The damage threshold (in terms of intensity or fluence) constitutes an upper limit for the operation parameters.

When dealing with pulses, a fast saturable absorber is one with a recovery time well below the pulse duration, whereas a slow absorber is one with a recovery time well above the pulse duration. This means that the same device may be either a fast absorber or a slow absorber, depending on the pulses with which it is used. A fast absorber is not necessarily better suited e.g. for passive mode locking; in fact, self-starting mode locking is more easily achieved with a slow absorber.

The saturation parameter of a saturable absorber (e.g. in a mode-locked laser) is the ratio of the incident pulse fluence to the saturation fluence of the device.

Selecting a Suitable Saturable Absorber

It depends very much on the concrete circumstances what properties of a saturable absorber are desirable. In particular, there are important differences between the requirements for Q switching and mode locking of lasers.

Typical requirements on a saturable absorber for a passively Q-switched laser are:

• The total non-saturated absorption must be relatively high – often slightly smaller than the small-signal gain of the laser medium, if a high pulse energy and short pulse duration is desired.
• A low saturation fluence and low non-saturable losses are desirable for minimizing the power losses.
• The recovery time should not be too long (although this problem occurs rarely). On the other hand, ideally it would also not be shorter than the pulse duration. The latter condition, however, is often not essential, particularly when the saturation fluence is far below the pulse fluence.
• The damage threshold in terms of intensity and fluence must be sufficiently high.

For passively mode-locked lasers, the requirements are different:

• The optimum modulation depth is typically quite small – often below 1%, and strongly depending on the type of laser. Tentatively, higher values are required for lasers with high resonator losses.
• The saturation fluence should usually be several times smaller than the pulse fluence under normal operation conditions. (The pulse fluence on the absorber may be adjusted via the beam radius resulting from the laser resonator design.)
• Depending on the mode locking mechanism used, the recovery time may or may not be important for achieving short pulses. For absorbers with a bitemporal response, the slow components may be useful for reliable self-starting characteristics.
• Low nonsaturable losses are again desirable for maximizing the laser's output power and efficiency.
• For avoiding damage of the absorber, the saturation conditions under normal operating conditions are usually of no concern. However, it can be essential to suppress Q-switching instabilities. Surprisingly, there are cases where absorber damage can be avoided by stronger focusing of the intracavity beam on the absorber, because this helps to suppress Q-switching instabilities. In some cases, particularly for high powers and for high pulse repetition rates, heating may be a concern.

Generally, decisions on absorber parameters should be made in the context of a comprehensive laser design processes, which takes into account both the dynamics of pulse generation and the limited tolerance of the absorber to high intensities or pulse energies.

Bibliography

See also: semiconductor saturable absorber mirrors, passive mode locking, mode-locked lasers, Q switching, Q-switched lasers, gain saturation

Categories: nonlinear optics, photonic devices, pulses