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Optical Clocks

Definition: time measurement devices based on optical frequency standards

German: optische Uhren

Categories: photonic devicesphotonic devices, optical metrologyoptical metrology

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Cite the article using its DOI: https://doi.org/10.61835/174

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An optical clock is a clock the output of which is derived from an optical frequency standard. As explained in the article on optical frequency standards, such a reference is based on atoms or ions which are kept in an optical trap and subject to laser cooling in order to suppress Doppler broadening. Their transition frequency is probed with a frequency-stabilized laser, the emission frequency of which is precisely locked to the atomic transition. That ultrastable optical frequency is far too high for electronic counting of oscillation cycles. However, it can be precisely related to lower (microwave) frequencies via some kind of optical clockwork, which is nowadays normally based on a frequency comb, as explained below. The obtained relation between the optical and microwave frequencies is highly accurate, normally not allowing for any phase slips.

An optical clock can offer an extremely high frequency precision and stability, far exceeding the performance of the best cesium atomic clocks. As its output, one may use the stabilized microwave frequency, the stable laser frequency or any of the spectral lines of the generated frequency comb. All those frequencies are highly stable, but the optical frequencies are more useful in the sense that precise frequency comparisons can be done within much shorter measurement times for such high frequencies.

Modern Optical Clockworks

In the early years of optical clocks, a severe challenge was to relate the stable optical frequency to a microwave frequency standard such as a cesium atomic clock: the required optical clockworks, at that time realized as frequency chains, were very difficult to make, and were applicable only to certain isolated optical frequencies. From 1999 on, however, very much simpler and much more versatile while equally precise optical clockworks have been realized on the basis of frequency combs from femtosecond mode-locked lasers [2].

setup of optical clock
Figure 1: Schematic setup of an optical clock.

A time signal is generated by a cesium clock. An optical frequency standard is used for reducing the long-term drift of the cesium clock. The frequency comparison is done using an optical clockwork. That clockwork may also provide an optical output, e.g. in the form of a frequency comb, allowing frequency comparison with other optical standards.

Comparison with Microwave Frequency Standards

Optical clocks are of interest not only for measuring optical frequencies, but also for general timekeeping where ultimate precision is required. Compared with microwave standards such as cesium atomic clocks, they have the following key advantages:

  • There are certain atoms and ions with extremely well-defined clock transitions (forbidden transitions) which promise higher accuracy and stability than the best microwave atomic clocks. The anticipated (but not yet demonstrated) relative frequency uncertainty of atomic optical clocks using electronic transitions is of the order of 10−18 for long enough averaging times (possibly a few days). It may even become possible to use certain low-energy nuclear transitions in order to get to 10−19 level [11].
  • The high optical frequencies themselves are of high importance because these allow precise clock comparisons within much shorter times. For example, a 10−15 precision can be achieved in a few seconds if the compared frequencies are in the optical range (hundreds of terahertz), whereas the order of a full day would be required with microwave clocks.
  • Optical signals can be easily transported over long distances using optical fibers. It is even possible to obtain a very precise time comparison between different clocks at different positions, using optical-frequency transfer over fiber-optic links [12]. Compared with fibers, microwave cables are more expensive and have much higher losses, and are therefore technically much more limited.

Redefining the Second

Because of the advantages of optical clocks in terms of accuracy, speed of comparison and remote synchronization, it is to be expected that in the not too far future the cesium clock as the fundamental timing reference will be replaced with an optical clock. This will effectively mean that the second as a fundamental SI unit will be redefined based on such a clock, then referring to an optical frequency rather than to a microwave frequency.

However, it is so far not clear which type of optical clock would be used as such a standard. A lattice clock [8] appears to be a good candidate, but the best choice of a particular clock atom is not obvious. Many criteria need to be considered. One of those is that the accuracy should be improved substantially (probably by about two orders of magnitude), but others are related to various practical aspects.

Even after that profound change, cesium clocks (and other non-optical atomic clocks, such as rubidium clocks) will continue to play an important role in technological applications as they can be simpler and more compact than optical clocks.

Video 1: This video on optical clocks has been provided by Menlo Systems.

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Bibliography

[1]N. V. Goldovskaya et al., “Possibility of establishment of a quantum frequency standard for the visible range using an intercombination spectral transition in the ytterbium atom”, Sov. J. Quantum Electron. 12 (12), 1659 (1982); https://doi.org/10.1070/QE1982v012n12ABEH006318
[2]S. A. Diddams et al., “Direct link between microwave and optical frequencies with a 300 THz femtosecond laser comb”, Phys. Rev. Lett. 82 (18), 3568 (1999); https://doi.org/10.1103/PhysRevLett.82.3568
[3]S. A. Diddams et al., “An optical clock based on a single trapped 199Hg+ ion”, Science 293, 825 (2001); https://doi.org/10.1126/science.1061171
[4]R. Holzwarth et al., “Optical clockworks and the measurement of laser frequencies with a mode-locked frequency comb”, IEEE J. Quantum Electron. 37 (12), 1493 (2001); https://doi.org/10.1109/3.970894
[5]T. Udem et al., “Optical frequency metrology”, Nature 416, 233 (2002); https://doi.org/10.1038/416233a
[6]L.-S. Ma et al., “Optical frequency synthesis and comparison with uncertainty at the 10−19 level”, Science 303, 1843 (2004); https://doi.org/10.1126/science.1095092
[7]S. A. Diddams et al., “Standards of time and frequency at the outset of the 21st century”, Science 306, 1318 (2004); https://doi.org/10.1126/science.1102330
[8]M. Takamoto et al., “An optical lattice clock”, Nature 435, 321 (2005); https://doi.org/10.1038/nature03541
[9]A. D. Ludlow et al., “Sr lattice clock at 1 × 10−16 fractional uncertainty by remote optical evaluation with a Ca clock”, Science Express Feb. 14, 2008; https://doi.org/10.1126/science.1153341
[10]C. W. Chou et al., “Frequency comparison of two high-accuracy Al+ optical clocks”, Phys. Rev. Lett. 104 (7), 070802 (2010); https://doi.org/10.1103/PhysRevLett.104.070802
[11]C. J. Campbell et al., “Single-ion nuclear clock for metrology at the 19th decimal place”, Phys. Rev. Lett. 108 (12), 120802 (2012); https://doi.org/10.1103/PhysRevLett.108.120802
[12]S. Droste et al., “Optical-frequency transfer over a singe-span 1840 km fiber link”, Phys. Rev. Lett. 111 (11), 110801 (2013); https://doi.org/10.1103/PhysRevLett.111.110801
[13]B. J. Bloom et al., “A new generation of atomic clocks: accuracy and stability at the 10−18 level”, http://arxiv.org/abs/1309.1137 (2013)
[14]A. D. Ludlow et al., “Optical atomic clocks”, arXiv:1407.3493v2
[15]F. Riehle, “Optical clock networks”, Nature Photon. 11, 25 (2017); https://doi.org/10.1038/nphoton.2016.235
[16]W. F. McGrew et al., “Towards the optical second: verifying optical clocks at the SI limit”, Optica 6 (4), 448 (2019); https://doi.org/10.1364/OPTICA.6.000448
[17]S. Herbers et al., “Transportable clock laser system with an instability of 1.6 × 10−16”, Opt. Lett. 47 (20), 5441 (2022); https://doi.org/10.1364/OL.470984

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Questions and Comments from Users

2022-05-13

Is the cesium clock still necessary? What if we defined the second based on the optical frequency standard in the diagram?

The author's answer:

Indeed, the second will eventually be redefined based on an optical frequency standard. Cesium clocks will then still be needed for various purposes, but often in conjunction with an optical frequency standard and an optical clockwork.

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